TY - JOUR
T1 - Harnessing structural darkness in the visible and infrared wavelengths for a new source of light
AU - Huang, Jianfeng
AU - Liu, Changxu
AU - Zhu, Yihan
AU - Masala, Silvia
AU - Alarousu, Erkki
AU - Han, Yu
AU - Fratalocchi, Andrea
N1 - Funding information:
This work is part of the Kaust research programme ‘Optics and plasmonics for efficient energy harvesting’, supported by award no. CRG-1-2012-FRA-005. Y.H. acknowledges baseline support funds from Kaust.
PY - 2016/1
Y1 - 2016/1
N2 - Engineering broadband light absorbers is crucial to many applications, including energy-harvesting devices and optical interconnects. The performances of an ideal absorber are that of a black body, a dark material that absorbs radiation at all angles and polarizations. Despite advances in micrometre-thick films, the absorbers available to date are still far from an ideal black body. Here, we describe a disordered nanostructured material that shows an almost ideal black-body absorption of 98–99% between 400 and 1,400 nm that is insensitive to the angle and polarization of the incident light. The material comprises nanoparticles composed of a nanorod with a nanosphere of 30 nm diameter attached. When diluted into liquids, a small concentration of nanoparticles absorbs on average 26% more than carbon nanotubes, the darkest material available to date. By pumping a dye optical amplifier with nanosecond pulses of ∼100 mW power, we harness the structural darkness of the material and create a new type of light source, which generates monochromatic emission (∼5 nm wide) without the need for any resonance. This is achieved through the dynamics of light condensation in which all absorbed electromagnetic energy spontaneously generates single-colour energy pulses.
AB - Engineering broadband light absorbers is crucial to many applications, including energy-harvesting devices and optical interconnects. The performances of an ideal absorber are that of a black body, a dark material that absorbs radiation at all angles and polarizations. Despite advances in micrometre-thick films, the absorbers available to date are still far from an ideal black body. Here, we describe a disordered nanostructured material that shows an almost ideal black-body absorption of 98–99% between 400 and 1,400 nm that is insensitive to the angle and polarization of the incident light. The material comprises nanoparticles composed of a nanorod with a nanosphere of 30 nm diameter attached. When diluted into liquids, a small concentration of nanoparticles absorbs on average 26% more than carbon nanotubes, the darkest material available to date. By pumping a dye optical amplifier with nanosecond pulses of ∼100 mW power, we harness the structural darkness of the material and create a new type of light source, which generates monochromatic emission (∼5 nm wide) without the need for any resonance. This is achieved through the dynamics of light condensation in which all absorbed electromagnetic energy spontaneously generates single-colour energy pulses.
U2 - 10.1038/nnano.2015.228
DO - 10.1038/nnano.2015.228
M3 - Article
SN - 1748-3387
VL - 11
SP - 60
EP - 66
JO - Nature Nanotechnology
JF - Nature Nanotechnology
IS - 1
ER -