How to go beyond C1 products with electrochemical reduction of CO2

Da Li, Hao Zhang, Hang Xiang, Shahid Rasul, Jean-Marie Fontmorin, Paniz Izadi, Alberto Roldan, Rebecca Taylor, Yujie Feng, Liam Banerji, Alexander Cowan*, Eileen H. Yu*, Jin Xuan*

*Corresponding author for this work

Research output: Contribution to journalReview articlepeer-review

4 Citations (Scopus)
23 Downloads (Pure)

Abstract

The electrochemical reduction of CO2 to produce fuels and value-added organic chemicals is of great potential, providing a mechanism to convert and store renewable energy within a carbon-neutral energy circle. Currently the majority of studies report C1 products such as carbon monoxide and formate as the major CO2 reduction products. A particularly challenging goal within CO2 electrochemical reduction is the pursuit of multi-carbon (C2+) products which have been proposed to enable a more economically viable value chain. This review summaries recent development across electro-, photoelectro- and bioelectro-catalyst developments. It also explores the role of device design and operating conditions in enabling C–C bond generation.
Original languageEnglish
Pages (from-to)5893-5914
Number of pages22
JournalSustainable Energy and Fuels
Volume5
Issue number23
Early online date20 Oct 2021
DOIs
Publication statusPublished - 7 Dec 2021

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